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Inverted organic solar cells with polymer-modified fluorine-doped tin oxide as the electron-collecting electrode

Identifieur interne : 000086 ( Main/Repository ); précédent : 000085; suivant : 000087

Inverted organic solar cells with polymer-modified fluorine-doped tin oxide as the electron-collecting electrode

Auteurs : RBID : Pascal:14-0091073

Descripteurs français

Pascal (Inist)
- Cellule solaire, Polymère, Addition fluor, Addition étain, Amine, Travail sortie, Sonde Kelvin, Thiophène, Butyrique dérivé polymère, Densité courant, Eclairement, Désorption, Substrat oxyde d'indium et de zinc, Substrat verre, 8460J, 7330.
Wicri :
- concept : Polymère.

English descriptors

KwdEn :
- Amine, Butyric derivative polymer, Current density, Desorption, Fluorine addition, Illumination, Kelvin probe, Polymer, Solar cell, Thiophene, Tin addition, Work function.

Abstract

We report on inverted solar cells using amine-containing polymer (polyethylenimine ethoxylated, PEIE) modified fluorine-doped tin oxide (FTO) as the electron-collecting electrode. PEIE lowers the work function of FTO from 4.6 eV to 3.8 eV, measured by Kelvin probe, sufficiently low for collecting electrons in solar cells. With the FTO/ PEIE electrode, inverted solar cells based on poly[(4,8-bis-(2-ethylhexyloxy)-benzo[1,2-b:4,5-b']dithiophene)-2,6-diyl-alt-(4-(2-ethylhexanoyl)-thieno[3,4-b]thiophene)-2,6-diyl]:phenyl-C₆₁-butyric acid methyl ester exhibited an open-circuit voltage of 0.70 ± 0.01 V, a short-circuit current density of 15.2 ± 0.2 mA/cm², a fill factor of 0.60 ± 0.01 and a power conversion efficiency of 6.3 ± 0.2% averaged over 9 devices under 100 mW/cm²AM1.5 illumination, which is comparable to the solar cells fabricated on indium-tin oxide glass substrates. In addition, we found that ultraviolet light-containing illumination can reduce the work function of bare FTO from 4.66 eV to 4.34 eV presumably because of the desorption of oxygen trapped in FTO.

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Pascal:14-0091073

Le document en format XML

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<author><name>JAE WON SHIM</name>
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<s2>Atlanta, GA 30332</s2>
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<author><name sortKey="Fuentes Hernandez, Canek" uniqKey="Fuentes Hernandez C">Canek Fuentes-Hernandez</name>
<affiliation wicri:level="4"><inist:fA14 i1="01"><s1>Center for Organic Photonics and Electronics (COPE), School of Electrical and Computer Engineering, Georgia Institute of Technology</s1>
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<author><name sortKey="Khan, Talha M" uniqKey="Khan T">Talha M. Khan</name>
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<author><name sortKey="Kippelen, Bernard" uniqKey="Kippelen B">Bernard Kippelen</name>
<affiliation wicri:level="4"><inist:fA14 i1="01"><s1>Center for Organic Photonics and Electronics (COPE), School of Electrical and Computer Engineering, Georgia Institute of Technology</s1>
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<term>Desorption</term>
<term>Fluorine addition</term>
<term>Illumination</term>
<term>Kelvin probe</term>
<term>Polymer</term>
<term>Solar cell</term>
<term>Thiophene</term>
<term>Tin addition</term>
<term>Work function</term>
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<keywords scheme="Pascal" xml:lang="fr"><term>Cellule solaire</term>
<term>Polymère</term>
<term>Addition fluor</term>
<term>Addition étain</term>
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<term>Travail sortie</term>
<term>Sonde Kelvin</term>
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<term>Butyrique dérivé polymère</term>
<term>Densité courant</term>
<term>Eclairement</term>
<term>Désorption</term>
<term>Substrat oxyde d'indium et de zinc</term>
<term>Substrat verre</term>
<term>8460J</term>
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<front><div type="abstract" xml:lang="en">We report on inverted solar cells using amine-containing polymer (polyethylenimine ethoxylated, PEIE) modified fluorine-doped tin oxide (FTO) as the electron-collecting electrode. PEIE lowers the work function of FTO from 4.6 eV to 3.8 eV, measured by Kelvin probe, sufficiently low for collecting electrons in solar cells. With the FTO/ PEIE electrode, inverted solar cells based on poly[(4,8-bis-(2-ethylhexyloxy)-benzo[1,2-b:4,5-b']dithiophene)-2,6-diyl-alt-(4-(2-ethylhexanoyl)-thieno[3,4-b]thiophene)-2,6-diyl]:phenyl-C<sub>61</sub>
-butyric acid methyl ester exhibited an open-circuit voltage of 0.70 ± 0.01 V, a short-circuit current density of 15.2 ± 0.2 mA/cm<sup>2</sup>
, a fill factor of 0.60 ± 0.01 and a power conversion efficiency of 6.3 ± 0.2% averaged over 9 devices under 100 mW/cm<sup>2 </sup>
AM1.5 illumination, which is comparable to the solar cells fabricated on indium-tin oxide glass substrates. In addition, we found that ultraviolet light-containing illumination can reduce the work function of bare FTO from 4.66 eV to 4.34 eV presumably because of the desorption of oxygen trapped in FTO.</div>
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<fC01 i1="01" l="ENG"><s0>We report on inverted solar cells using amine-containing polymer (polyethylenimine ethoxylated, PEIE) modified fluorine-doped tin oxide (FTO) as the electron-collecting electrode. PEIE lowers the work function of FTO from 4.6 eV to 3.8 eV, measured by Kelvin probe, sufficiently low for collecting electrons in solar cells. With the FTO/ PEIE electrode, inverted solar cells based on poly[(4,8-bis-(2-ethylhexyloxy)-benzo[1,2-b:4,5-b']dithiophene)-2,6-diyl-alt-(4-(2-ethylhexanoyl)-thieno[3,4-b]thiophene)-2,6-diyl]:phenyl-C<sub>61</sub>
-butyric acid methyl ester exhibited an open-circuit voltage of 0.70 ± 0.01 V, a short-circuit current density of 15.2 ± 0.2 mA/cm<sup>2</sup>
, a fill factor of 0.60 ± 0.01 and a power conversion efficiency of 6.3 ± 0.2% averaged over 9 devices under 100 mW/cm<sup>2 </sup>
AM1.5 illumination, which is comparable to the solar cells fabricated on indium-tin oxide glass substrates. In addition, we found that ultraviolet light-containing illumination can reduce the work function of bare FTO from 4.66 eV to 4.34 eV presumably because of the desorption of oxygen trapped in FTO.</s0>
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Inverted organic solar cells with polymer-modified fluorine-doped tin oxide as the electron-collecting electrode

Inverted organic solar cells with polymer-modified fluorine-doped tin oxide as the electron-collecting electrode

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